According to support and https://help.blackboard.com/Learn/Student/Interact/Organizations it is not possible for a participant to self-unenrol from an organization. You can let them self-enrol but once they're in there, their only way out is contacting the Leaders or administrators.
We would like to have an organization for the student union where all students are automatically enrolled but can choose to leave if they so please, a sort of "opt-out" approach. Without self-unenrol, this is not possible.
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